On the rules screen, it would be good if you could browse to the files and folders to select them rather than having to type them in.
New: Run-Command (Dec 2, 2024), Platform 29.5.3 (Jun 27, 2024)
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you create a set of rules and then select then in a tab (i.e. Sync, Backup or Secure) you can right click on files and folders you have added and exclude them there.